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Science · Chemistry

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Synthesis of covalent organic frameworks for photocatalytic hydrogen peroxide production guided by large language models

The photosynthetic production of hydrogen peroxide (H2O2) from water and oxygen presents a sustainable alternative to the energy-intensive anthraquinone process. Covalent organic frameworks (COFs) have emerged as promising photocatalysts for H2O2 generation. However, most existing COF photocatalysts yield H2O2 at concentrations too low for practical applications, largely due to ongoing challenges in simultaneously optimizing photocatalytic activity and structural stability. Here, we introduce a large language mo…

Nature Communications · Science

Synthesis of covalent organic frameworks for photocatalytic hydrogen peroxide production guided by large language models